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You are researching: Polyphenylene Oxide
Cell Type
Tissue and Organ Biofabrication
Skin Tissue Engineering
Drug Delivery
Biological Molecules
Solid Dosage Drugs
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AUTHOR
Title
3D-printed monolithic porous adsorbents from a solution-processible, hypercrosslinkable, functionalizable polymer
[Abstract]
Year
2021
Journal/Proceedings
Chemical Engineering Journal
Reftype
Groups
AbstractSolid adsorbents have been actively developed for energy-efficient gas separations including carbon capture and air purification. However, conventional particulate adsorbents often show ineffective mass transfer and significant pressure drop in practical operations, leading to a limited overall performance. As a potential solution to these issues, the development of three-dimensionally (3D) structured adsorbents has been proposed. Herein, we report a novel approach to design 3D monolithic adsorbents for CO2 separation via 3D printing of a processible polymer, which in turn can be transformed into a functional porous material via hypercrosslinking and amine-grafting. Importantly, such structure can be realized without an aid from binders or mechanical supports. Our adsorbents demonstrated a promising CO2 adsorption performance without experiencing any pressure drop under dynamic flow condition. The stability and regenerability, which are also important requirements for practical operations, were also successfully demonstrated through a repetitive adsorption-desorption cycling test in the presence of water vapor. We envisage that our approach can be applied in the development of structurally versatile adsorbents for various gas separation processes.